Subido por Chandan Prasad Kushwaha

Chandan Abstract (1)

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TEMPERATURE-DEPENDENT PHOTOLUMINESCENCE STUDIES OF TMDC
HETEROBILAYERS: TOWARDS MOIRE EXCITONS
The discovery of superconductivity in the twisted graphene bilayers with a 1.1-degree twist
angle (the magic angle), has led to a significant interest in twisted 2D material.1 On twisting
two transition metal dichalcogenide (TMDC) mono-layers relative to one another, the natural
periodic potential arising from the atomic cores can be altered, and the new periodicity gives
rise to the Moire potentials.2 Optically, it manifests as the fine splitting in the
photoluminescence (PL) spectra.3 Since the lattice mismatch condition is relaxed in these Van
der Waals materials, it provides an efficient and relatively simple approach for tuning the band
properties of emergent TMDC heterostructures.4 In the present work, we present the study of
temperature-dependent PL in three bilayer systems, namely: MoWSe2/MoSe2, MoS2/MoSe2
and in near-zero degree twisted MoSe2/MoSe2 homo-bilayer. From a detailed analysis, we
extract the temperature-dependent parameters of these heterostructures. The MoSe2/MoSe2
zero-degree twisted bilayer exhibits optical features pointing towards the Moire excitons.
Future pump-probe transient reflectance studies will shed light on the Moire exciton dynamics
in these twisted bilayer systems.
References:
1.
Devakul, Trithep, et al. "Magic in twisted transition metal dichalcogenide
bilayers." Nature communications 12.1 (2021): 6730.
2.
Marcellina, Elizabeth, et al. "Evidence for moiré trions in twisted MoSe2
homobilayers." Nano Letters 21.10 (2021): 4461-4468.
3.
Zhang, Nan, et al. "Moiré intralayer excitons in a MoSe2/MoS2 heterostructure." Nano
letters 18.12 (2018): 7651-7657.
4.
Villafañe, Viviana, et al. "Twist-Dependent Intra-and Interlayer Excitons in Moiré
MoSe2 Homobilayers." Physical Review Letters 130.2 (2023): 026901.
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